Spatial variability, source identification and risks assessment of antibiotics in multimedia of North China's largest freshwater lake using positive matrix factorization and Monte Carlo simulation

Primer Autor
Bai, Junhong
Co-autores
Zhang, Ling
Zhang, Kegang
Zhai, Yujia
Wang, Yaqi
Liu, Haizhu
Xiao, Rong
Jorquera, Milko A.
Xia, Jiangbao
Título
Spatial variability, source identification and risks assessment of antibiotics in multimedia of North China's largest freshwater lake using positive matrix factorization and Monte Carlo simulation
Editorial
ELSEVIER
Revista
JOURNAL OF HAZARDOUS MATERIALS
Lenguaje
en
Resumen
Antibiotics are widely found in aquatic ecosystems and pose a serious threat to human and the ecological system. Samples of surface water (SW), overlying water (OW), pore water (PW) and sediments (Sedi) were collected to investigate the spatial variability, potential sources, ecological risk (RQs) and health risks (HQs) of nine common antibiotics in Baiyangdian Lake using positive matrix factorization (PMF), and Monte Carlo simulation. Signif-icant spatial autocorrelation of most antibiotics were observed in PW and Sedi samples rather than in SW and OW samples, and higher antibiotic levels were found in the northwest of waters and the southwest of sediments. Livestock (26.74-35.57%) and aquaculture (21.62-37.70%) were identified as primary sources of antibiotics in the water and sediments. Norfloxacin and roxithromycin showed high levels of RQ and HQ in more than 50% of samples, respectively. The combined RQ (& sigma,RQ) in the PW can be used as a sign of across multimedia risk. Notably, appreciable health risks were observed for the combined HQ (& sigma,HQ) in about 80% of samples, indicating the importance of taking health risk of antibiotics into consideration. The findings of this work provides a reference for antibiotics pollution control and risk management in shallow lake.
Fecha Publicación
2023
Tipo de Recurso
artículo original
doi
10.1016/j.jhazmat.2023.131751
Formato Recurso
PDF
Palabras Claves
Antibiotics
Spatial variability
Source identification
Risk assessment
Shallow lake
Ubicación del archivo
Categoría OCDE
Ingeniería
Ciencias Ambientales y Ecología
Materias
Antibióticos
variabilidad espacial
Identificación de fuente
Evaluación de riesgos
lago poco profundo
Identificador del recurso (Mandatado-único)
artículo original
Versión del recurso (Recomendado-único)
versión publicada
Derechos de acceso
metadata
Access Rights
metadata
Id de Web of Science
WOS:001012314500001
ISSN
0304-3894
Tipo de ruta
hibrida
Categoría WOS
Ingeniería
Ciencias Ambientales y Ecología
Referencia del Financiador (Mandatado si es aplicable-repetible)
NSFC 51961125201
ANID NSFC190012
ANID 190012
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